Intercomparison of in situ measurements of ambient NH-3: instrument performance and application under field conditions

Twigg, Marsailidh M.; Berkhout, Augustinus J.C.; Cowan, Nicholas; Crunaire, Sabine; Dammers, Enrico; Ebert, Volker; Gaudion, Vincent; Haaima, Marty; Häni, Christoph; John, Lewis; Jones, Matthew R.; Kamps, Bjorn; Kentisbeer, John; Kupper, Thomas; Leeson, Sarah R.; Leuenberger, Daiana; Lüttschwager, Nils O. B.; Makkonen, Ulla; Martin, Nicholas A.; Missler, David; Mounsor, Duncan; Neftel, Albrecht; Nelson, Chad; Nemitz, Eiko; Oudwater, Rutger; Pascale, Celine; Petit, Jean-Eudes; Pogány, Andrea; Redon, Nathalie; Sintermann, Jörg; Stephens, Amy; Sutton, Mark A.; Tang, Yuk S.; Zijlmans, Rens; Braban, Christine F.; Niederhauser, Bernhard

doi:https://doi.org/10.5194/amt-2022-107

Zugriffsnummer	48744
Dokumenttyp	Zeitschriftenartikel
Peer Review	mit Peer Review
Sprache	Englisch
Titel	Intercomparison of in situ measurements of ambient NH-3: instrument performance and application under field conditions
Autor(in); Institution	Twigg, Marsailidh M.; UK Centre for Ecology & Hydrology, Penicuik, UK Berkhout, Augustinus J.C.; National Institute for Public Health and the Environment (RIVM), Bilthoven, THE NETHERLANDS Cowan, Nicholas; UK Centre for Ecology & Hydrology, Penicuik, UK Crunaire, Sabine; Université Lille, Lille, FRANCE Dammers, Enrico; TNO, Utrecht, THE NETHERLANDS Ebert, Volker; 3.4, Analytische Chemie der Gasphase, PTB-Braunschweig Gaudion, Vincent; Université Lille, Lille, FRANCE Haaima, Marty; National Institute for Public Health and the Environment (RIVM), Bilthoven, THE NETHERLANDS Häni, Christoph; Bern University of Applied Sciences, Zollikofen, SWITZERLAND John, Lewis; Enviro Technology Services Ltd, UK Jones, Matthew R.; UK Centre for Ecology & Hydrology, Penicuik, UK Kamps, Bjorn; LSE monitors BV, THE NETHERLANDS Kentisbeer, John; UK Centre for Ecology & Hydrology, Penicuik, UK Kupper, Thomas; Bern University of Applied Sciences, Zollikofen, SWITZERLAND Leeson, Sarah R.; UK Centre for Ecology & Hydrology, Penicuik, UK Leuenberger, Daiana; Federal Institute of Metrology (METAS), Bern-Wabern, SWITZERLAND Lüttschwager, Nils O. B.; 3.4, Analytische Chemie der Gasphase, PTB-Braunschweig Makkonen, Ulla; Finnish Meteorological Institute, Helsinki, FINLAND Martin, Nicholas A.; National Physical laboratory, Teddington, UK Missler, David; Atmo Grand-Est, Schiltigheim, FRANCE Mounsor, Duncan; Enviro Technology Services Ltd, UK Neftel, Albrecht; Neftel Research Expertise, SWITZERLAND Nelson, Chad; Tiger Optics, USA Nemitz, Eiko; UK Centre for Ecology & Hydrology, Penicuik, UK Oudwater, Rutger; Tiger Optics, USA Pascale, Celine; Federal Institute of Metrology (METAS), Bern-Wabern, SWITZERLAND Petit, Jean-Eudes; Laboratoire des Sciences du Climat et de l'Environnement, CEA, Gif-sur-Yvette, FRANCE Pogány, Andrea; 3.4, Analytische Chemie der Gasphase, PTB-Braunschweig Redon, Nathalie; Université Lille, Lille, FRANCE Sintermann, Jörg; Office of Waste, Water, Energy and Air AWEL, Zürich, SWITZERLAND Stephens, Amy; UK Centre for Ecology & Hydrology, Penicuik, UK Sutton, Mark A.; UK Centre for Ecology & Hydrology, Penicuik, UK Tang, Yuk S.; UK Centre for Ecology & Hydrology, Penicuik, UK Zijlmans, Rens; LSE monitors BV, THE NETHERLANDS Braban, Christine F.; UK Centre for Ecology & Hydrology, Penicuik, UK Niederhauser, Bernhard; Federal Institute of Metrology (METAS), Bern-Wabern, SWITZERLAND
Quelle/Jahr	Atmospheric Measurement Techniques Discussions:(2022), 6755 - 6787
Availability	[online only]
ISSN	1867-8610 (online)
DOI	https://doi.org/10.5194/amt-2022-107 https://doi.org/10.5194/amt-15-6755-2022
Verlag	Katlenburg-Lindau: Copernicus
Zusammenfassung	Ammonia (NH3) in the atmosphere affects both the environment and human health. It is therefore increasingly recognised by policy makers as an important air pollutant that needs to be mitigated. In order to understand the effectiveness of abatement strategies, routine NH3 monitoring is required. Current reference protocols, developed in the 1990s, use daily samplers with offline analysis but there have been a number of technologies developed since, which may be applicable for high time resolution routine monitoring of NH3 at ambient concentrations. The following study is a comprehensive field intercomparison held over an intensively managed grassland in South East Scotland using currently available methods that are reported to be suitable for routine monitoring of ambient NH3. In total 13 instruments took part in the field study. The instruments include: an online ion chromatography system (MARGA, Metrohm-Applikon,NL), two wet chemistry continuous flow analysis systems (AiRRmonia, Mechatronics, NL), a photoacoustic spectrometer (NH3 monitor, LSE, NL), two mini Differential Optical Absorption Spectrometers (miniDOAS; NTB Interstate University of Applied Sciences Buchs, now part of "Eastern Switzerland University of Applied Sciences, CH and RIVM, NL), as well as seven spectrometers using cavity enhanced techniques: a Quantum Cascade Laser Absorption Spectrometer (QCLAS, Aerodyne, Inc. US), Picarro G2103 Analyzer (Picarro US), Economical NH3 Analyser (Los Gatos Research, US), Tiger-i 2000 (Tiger Optics, US) and LaserCEM® gas analyser (AP2E, FR).

Kostenfreier Zugang	Open Access Gold
Rechteinformation	CC BY 4.0 ; Creative Commons Attribution 4.0 License

Förderinformationen (1)	Förderername: European Commission (EC) Förderer ID: 0000 0001 2242 8989 Förderer ID Typ: ISNI Förderprogramm: EMPIR 2013 Environment Titel der Förderung: ENV55: MetNH3: Metrology for ammonia in ambient air Förderungsnummer: ENV55
Förderinformationen (2)	Förderername: Natural Environment Research Council (NERC) Förderer ID: 0000 0001 2181 0377 Förderer ID Typ: ISNI Förderungsnummer: NE/R016429/1
Förderinformationen (3)	Förderername: Natural Environment Research Council (NERC) Förderer ID: 0000 0001 2181 0377 Förderer ID Typ: ISNI Förderungsnummer: NE/T001798/1
Förderinformationen (4)	Förderername: Bundesamt für Umwelt (BAFU) Förderer ID: 0000 0001 1271 413X Förderer ID Typ: ISNI Förderungsnummer: 06.9115.P2IP246-1000
Förderinformationen (5)	Förderername: French Ministry of Environment Förderungsnummer: 2200995403

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Twigg, M. M., Berkhout, A. J., Cowan, N., Crunaire, S., Dammers, E., Ebert, V., Gaudion, V., Haaima, M., Häni, C., John, L., Jones, M. R., Kamps, B., Kentisbeer, J., Kupper, T., Leeson, S. R., Leuenberger, D., Lüttschwager, N. O. B., Makkonen, U., Martin, N. A., Missler, D., Mounsor, D., Neftel, A., Nelson, C., Nemitz, E., Oudwater, R., Pascale, C., Petit, J.-E., Pogány, A., Redon, N., Sintermann, J., Stephens, A., Sutton, M. A., Tang, Y. S., Zijlmans, R., Braban, C. F., & Niederhauser, B. (2022). Intercomparison of in situ measurements of ambient NH-3: instrument performance and application under field conditions. Atmospheric Measurement Techniques Discussions, 6755–6787. https://doi.org/10.5194/amt-2022-107

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