Zugriffsnummer 41847
Dokumenttyp Zeitschriftenartikel
Peer Review mit Peer Review
Sprache Englisch
Titel Probing the structural transition from buffer layer to quasifreestanding monolayer graphene by Raman spectroscopy
Autor(in); Institution
Wundrack, Stefan; 3.1, Allgemeine und Anorganische Chemie, PTB-Braunschweig
Momeni Pakdehi, Davood; 2.5, Halbleiterphysik und Magnetismus, PTB-Braunschweig
Schädlich, P.; Technische Universität Chemnitz, Institut für Physik, Chemnitz, GERMANY
Speck, F.; Technische Universität Chemnitz, Institut für Physik, Chemnitz, GERMANY
Pierz, K.; 2.5, Halbleiterphysik und Magnetismus, PTB-Braunschweig
Seyller, T.; Technische Universität Chemnitz, Institut für Physik, Chemnitz, GERMANY
Schumacher, Hans Werner; 2.5, Halbleiterphysik und Magnetismus, PTB-Braunschweig
Bakin, A.; TU Braunschweig, Institut für Halbleitertechnik, Braunschweig, GERMANY; TU Braunschweig, Laboratory of Emerging Nanometrology (LENA), Braunschweig, GERMANY
Stosch, Rainer; 3.1, Allgemeine und Anorganische Chemie, PTB-Braunschweig
Quelle/Jahr Physical Review B: 99 (2019), 4, 1 - 8
Artikelnummer 045443
ISSN 2469-9950 (PRINT) ; 2469-9969 (ONLINE)
DOI
Verlag Ridge, NY: American Physical Society (APS)
Zusammenfassung The structural transition of a graphene buffer layer epitaxially grown on 6H silicon carbide (SiC) to quasifreestanding monolayer graphene by intercalation of oxygen and water molecules at low concentrations is studied by temperature-dependent Raman spectroscopy. We present a detailed investigation of the defect density and strain and doping evolution in the graphene crystal lattice. The structural transition from the buffer layer to monolayer graphene with high defect densities occurs at temperatures from 400 to 500 °C, revealing the nanocrystalline regime of stage 2 of the amorphization trajectory, followed by the transition into stage 1 as evidenced by a gradual reduction of defects in graphene during subsequent annealing up to 900 °C.

Zitierung

Wundrack, S., Momeni Pakdehi, D., Schädlich, P., Speck, F., Pierz, K., Seyller, T., Schumacher, H. W., Bakin, A., & Stosch, R. (2019). Probing the structural transition from buffer layer to quasifreestanding monolayer graphene by Raman spectroscopy. Physical Review B, 99(4), 1–8. https://doi.org/10.1103/physrevb.99.045443

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